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- W2052008047 abstract "The conditions at which explosion is brought about in reacting systems of varying size and shape are investigated. The results are used to assess, for the first time, theoretical rules for scaling from laboratory tests, and predictions for the effect of shape. A gaseous substrate is used (ditertiary-butyl peroxide) and it is decomposed at pressuresless than 10 Torr and temperatures in the range 450–510 K. Heat transport is by conduction in these circumstances and when ignition occurs it is as a result of thermal runaway. Thus the behaviour of the system is analogous to that of many exothermic solids. The vessel shapes in which reaction was investigated include spheres, an oblate spheroid, cylinders and a toroid. The p-Ta ignition boundaries are established at different conditions in each of the vesselsand the need for a reliable means of quantifying these variations is thus exemplified. A procedure derived by Boddington, Gray and Harvey provides that route and it is validated by the normalization carried out in the present study. The need for exceptionally precise kinetic data is emphasized if the bounds for safe handling of materials are to be deduced without recourse to any experimental study." @default.
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- W2052008047 date "1982-01-01" @default.
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- W2052008047 title "Explosion hazards in exothermic materials: Critical conditions and scaling rules for masses of different geometry" @default.
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- W2052008047 doi "https://doi.org/10.1016/s0082-0784(82)80258-0" @default.
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