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• W2052051218 abstract "Two interesting features can normally be expected in the Raman spectrum of a molecule with a degenerate electronic ground state (i) the contribution of asymmetric or even antisymmetric tensors to the Raman intensity (ii) lifting of the electronic degeneracy due to Jahn-Teller distortion. The experimental data and discussion on VCl4, presented here, show that this molecule does not show any deviations in the Raman selection rules. Further, its Raman spectrum closely resembles that of TiCl4 which also has Td geometry but a nondegenerate singlet ground state. This suggests the absence of any static Jahn-Teller distortion in VCl4. However, we have observed a broadening of the ν2 band of VCl4 over TiCl4 and we attribute this to a possible dynamic Jahn-Teller splitting." @default.
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• W2052051218 date "1977-09-01" @default.
• W2052051218 modified "2023-10-18" @default.
• W2052051218 title "Selection rules and Raman spectrum of a molecule with a degenerate ground state and zero spin-orbit coupling: VCl4" @default.
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• W2052051218 doi "https://doi.org/10.1016/0022-2852(77)90293-4" @default.
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