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- W2052055251 abstract "The strengths of the $^{5}$${mathit{D}}_{0}$${mathrm{ensuremath{-}}}^{7}$${mathit{F}}_{mathit{J}}$ (J=0,2,4) optical transitions of the ${mathrm{Sm}}^{2+}$ ion in solids, which are due to the forced electric dipole transition, are analyzed by taking into account not only the Judd-Ofelt mechanism but also the excited-state spin-orbit interaction (Wybourne-Downer) mechanism. The fact that the $^{5}$${mathit{D}}_{0}$${mathrm{ensuremath{-}}}^{7}$${mathit{F}}_{0}$ transition strength of the ${mathrm{Sm}}^{2+}$ ion is much larger than that of the isoelectronic ${mathrm{Eu}}^{3+}$ ion in various crystalline and glassy matrices is ascribed to the resonance effect which results from the presence of the 4${mathit{f}}^{5}$5d states of ${mathrm{Sm}}^{2+}$ in the vicinity of the 4${mathit{f}}^{6}$ states concerned with the optical transition. However, such an enhancement of the transition strength due to the energetic resonance between the 4${mathit{f}}^{6}$ and 4${mathit{f}}^{5}$5d states is not observed in the $^{5}$${mathit{D}}_{0}$${mathrm{ensuremath{-}}}^{7}$${mathit{F}}_{2,4}$ transitions of ${mathrm{Sm}}^{2+}$ in solids. This is identified as due to the interference between the Judd-Ofelt and Wybourne-Downer mechanisms. textcopyright{} 1996 The American Physical Society." @default.
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