Matches in SemOpenAlex for { <https://semopenalex.org/work/W2052622204> ?p ?o ?g. }
- W2052622204 endingPage "77" @default.
- W2052622204 startingPage "68" @default.
- W2052622204 abstract "Decay of excited state absorption, owing to charge injection into the conduction band continuum of semiconductor states, is obtained via a qualitative theoretical model. The density matrix formalism is utilized to obtain an expression for the sequential pump−probe signal in terms of the nonlinear third-order polarization of the molecular system. Electron transfer slower than the pump and probe pulses is assumed and reorganization of the molecule upon charge injection is ignored while obtaining the final expressions. The lifetime of the excited state decouples from nuclear motion as a consequence. Decay of the excited state into a continuum of electronic states is examined for various energy positions of the injecting state and for different bandwidths of the continuum. The decay can be fitted by exponential functions for the majority of the cases considering different dimensionalities of the semiconductor continuum. Model calculations are performed for the snapshot limit of the pump−probe signal. Under the assumed conditions one obtains oscillations due to vibronic coherences that are superimposed on temperature-independent irreversible charge transfer decays, as is reported in recent experiments." @default.
- W2052622204 created "2016-06-24" @default.
- W2052622204 creator A5007826147 @default.
- W2052622204 creator A5036355702 @default.
- W2052622204 date "1999-12-09" @default.
- W2052622204 modified "2023-10-16" @default.
- W2052622204 title "Pump−Probe Spectroscopy of Ultrafast Electron Injection from the Excited State of an Anchored Chromophore to a Semiconductor Surface in UHV: A Theoretical Model" @default.
- W2052622204 cites W1971092996 @default.
- W2052622204 cites W1971472669 @default.
- W2052622204 cites W1973805557 @default.
- W2052622204 cites W1979726102 @default.
- W2052622204 cites W1980216394 @default.
- W2052622204 cites W1986723594 @default.
- W2052622204 cites W1987586480 @default.
- W2052622204 cites W2002256729 @default.
- W2052622204 cites W2012606475 @default.
- W2052622204 cites W2013998255 @default.
- W2052622204 cites W2020806697 @default.
- W2052622204 cites W2022022904 @default.
- W2052622204 cites W2023917857 @default.
- W2052622204 cites W2024485683 @default.
- W2052622204 cites W2026851119 @default.
- W2052622204 cites W2027045192 @default.
- W2052622204 cites W2036464008 @default.
- W2052622204 cites W2040881355 @default.
- W2052622204 cites W2043434510 @default.
- W2052622204 cites W2045989429 @default.
- W2052622204 cites W2048569527 @default.
- W2052622204 cites W2050764526 @default.
- W2052622204 cites W2052283301 @default.
- W2052622204 cites W2055069556 @default.
- W2052622204 cites W2059900987 @default.
- W2052622204 cites W2065845770 @default.
- W2052622204 cites W2068597378 @default.
- W2052622204 cites W2071188564 @default.
- W2052622204 cites W2073738597 @default.
- W2052622204 cites W2081673494 @default.
- W2052622204 cites W2087966232 @default.
- W2052622204 cites W2088208999 @default.
- W2052622204 cites W2093665937 @default.
- W2052622204 cites W2095323045 @default.
- W2052622204 cites W2141464177 @default.
- W2052622204 cites W2167558596 @default.
- W2052622204 cites W2173306066 @default.
- W2052622204 cites W2222517232 @default.
- W2052622204 cites W2478779981 @default.
- W2052622204 cites W2482810354 @default.
- W2052622204 cites W4231000464 @default.
- W2052622204 cites W780485881 @default.
- W2052622204 doi "https://doi.org/10.1021/jp991428r" @default.
- W2052622204 hasPublicationYear "1999" @default.
- W2052622204 type Work @default.
- W2052622204 sameAs 2052622204 @default.
- W2052622204 citedByCount "66" @default.
- W2052622204 countsByYear W20526222042012 @default.
- W2052622204 countsByYear W20526222042013 @default.
- W2052622204 countsByYear W20526222042014 @default.
- W2052622204 countsByYear W20526222042015 @default.
- W2052622204 countsByYear W20526222042016 @default.
- W2052622204 countsByYear W20526222042019 @default.
- W2052622204 countsByYear W20526222042020 @default.
- W2052622204 crossrefType "journal-article" @default.
- W2052622204 hasAuthorship W2052622204A5007826147 @default.
- W2052622204 hasAuthorship W2052622204A5036355702 @default.
- W2052622204 hasConcept C108225325 @default.
- W2052622204 hasConcept C121332964 @default.
- W2052622204 hasConcept C147120987 @default.
- W2052622204 hasConcept C178596936 @default.
- W2052622204 hasConcept C181500209 @default.
- W2052622204 hasConcept C184779094 @default.
- W2052622204 hasConcept C185592680 @default.
- W2052622204 hasConcept C32891209 @default.
- W2052622204 hasConcept C41999313 @default.
- W2052622204 hasConcept C520434653 @default.
- W2052622204 hasConcept C56911000 @default.
- W2052622204 hasConcept C62520636 @default.
- W2052622204 hasConcept C84114770 @default.
- W2052622204 hasConceptScore W2052622204C108225325 @default.
- W2052622204 hasConceptScore W2052622204C121332964 @default.
- W2052622204 hasConceptScore W2052622204C147120987 @default.
- W2052622204 hasConceptScore W2052622204C178596936 @default.
- W2052622204 hasConceptScore W2052622204C181500209 @default.
- W2052622204 hasConceptScore W2052622204C184779094 @default.
- W2052622204 hasConceptScore W2052622204C185592680 @default.
- W2052622204 hasConceptScore W2052622204C32891209 @default.
- W2052622204 hasConceptScore W2052622204C41999313 @default.
- W2052622204 hasConceptScore W2052622204C520434653 @default.
- W2052622204 hasConceptScore W2052622204C56911000 @default.
- W2052622204 hasConceptScore W2052622204C62520636 @default.
- W2052622204 hasConceptScore W2052622204C84114770 @default.
- W2052622204 hasIssue "1" @default.
- W2052622204 hasLocation W20526222041 @default.
- W2052622204 hasOpenAccess W2052622204 @default.
- W2052622204 hasPrimaryLocation W20526222041 @default.
- W2052622204 hasRelatedWork W1606781778 @default.
- W2052622204 hasRelatedWork W1971593760 @default.
- W2052622204 hasRelatedWork W1982518179 @default.
- W2052622204 hasRelatedWork W2068137917 @default.