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• W2052916422 abstract "Vibration–vibration energy exchange probabilities between iodine molecules (X 1Σ+g) have been calculated by use of the solution of the time-dependent Schrödinger equation. The interaction potential is constructed by summing four orientation averaged atom–atom interactions. One-quantum probabilities Pv,0v−1,1(T) for v−1,1→v,0 are found to be very large in a temperature range of 100–3000 K. At lower temperatures, the approximate linear relation pv,0v−1,1(T)≂vP1,00,1(T) holds. When v is small, the probability increases linearly with temperature. Multiquantum transitions v,0→v−n,n with n≳1 are found to be negligible near room temperature, but they become quite efficient at higher temperatures. Energy exchange probabilities are formulated in infinite order and their reduction to first-order expressions are discussed in detail. The effects of molecular attraction are also discussed." @default.
• W2052916422 created "2016-06-24" @default.
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• W2052916422 date "1983-02-01" @default.
• W2052916422 modified "2023-09-23" @default.
• W2052916422 title "Vibration–vibration energy exchange in iodine molecules" @default.
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• W2052916422 doi "https://doi.org/10.1063/1.444908" @default.
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