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• W2052942155 abstract "A novel palladium-catalyzed intramolecular oxidative aminofluorination of unactivated alkenes has been developed, in which AgF was used as a key fluorinating reagent and PhI(OPiv)2 as oxidant. The reaction afforded vicinal fluoroamine products with very high regioselectivity. A Pd(II/IV) catalytic cycle was proposed, and preliminary mechanistic studies indicated that direct reductive elimination of Pd(IV) intermediates is favored, albeit competing with SN2 nucleophilic attack by fluorine, to form a C−F bond." @default.
• W2052942155 created "2016-06-24" @default.
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• W2052942155 creator A5053353366 @default.
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• W2052942155 date "2009-10-26" @default.
• W2052942155 modified "2023-10-18" @default.
• W2052942155 title "Palladium-Catalyzed Intramolecular Aminofluorination of Unactivated Alkenes" @default.
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• W2052942155 doi "https://doi.org/10.1021/ja9076588" @default.
• W2052942155 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/19856929" @default.
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