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- W2053018338 abstract "Abstract To understand the carbon isotope fractionation during the mineral-catalyzed Fischer-Tropsch synthesis of hydrocarbons under hydrothermal conditions, experiments on formic acid were carried out at 300°C and 35 MPa using gold tubes in the presence of Fe as a catalyst. The experiments were composed of two groups: with and without water. Due to the limited volume of the gold tubes, only methane was available for isotopic analyses among all produced hydrocarbons. The results demonstrate that CO 2 is the gas most enriched in 13 C whereas methane is the gas most depleted in 13 C. Moreover, methane becomes more and more depleted in 13 C with an increase in reaction time. The carbon isotopic fractionation between CO 2 and CH 4 (α(CO 2 -CH 4 )) reached 1.052–1.059 at 144 h, which is similar to those of microbial reduction of CO 2 to CH 4 by methanogenic bacteria (1.048–1.079). This implies that carbon isotopic fractionation during Fischer-Tropsch synthesis is controlled by kinetic isotopic effects." @default.
- W2053018338 created "2016-06-24" @default.
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- W2053018338 date "2011-04-01" @default.
- W2053018338 modified "2023-09-27" @default.
- W2053018338 title "Carbon isotopic fractionations during Fischer-Tropsch synthesis" @default.
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- W2053018338 doi "https://doi.org/10.1016/s1876-3804(11)60031-1" @default.
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