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• W2053113685 abstract "We have performed molecular dynamics computer simulations of water in homogeneous external electric fields which were varied in a wide range of field strengths. The dielectric response is found to be linear up to fields E0≈0.01 V/Å from where dielectric saturation effects become important. At fields of E0≈3 V/Å a phase transition into an ordered, ice-like structure is observed, which is stabilized through hydrogen-bonds. With an increasing external electric field, the frequency spectrum of the water dynamics shows a remarkable red shift of the intramolecular modes and a blue shift of the librational motions, where the frequency varies quadratically with the field strength. A simple analytical model is discussed which reproduces the observed behavior." @default.
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• W2053113685 date "1998-06-01" @default.
• W2053113685 modified "2023-10-02" @default.
• W2053113685 title "Structure formation and dynamics of water in strong external electric fields" @default.
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• W2053113685 doi "https://doi.org/10.1016/s0022-0728(97)00649-9" @default.
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