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• W2053184447 abstract "Analytical expressions are provided for charged and uncharged particles in the perfect-wetting limit of Fletcher's classical heterogeneous nucleation theory with finite activation energy G*. A dimensionless logarithm of the critical supersaturation can be represented as a single universal curve versus a dimensionless nucleus radius for neutral particles, while a uniparametric family of curves is required for charged particles. Comparison with experimental critical supersaturations for nanoparticles and molecular ions shows qualitative agreement, with substantial quantitative disagreement. At increasing sizes the predicted critical diameter augmented by a fixed length ∼1 nm approaches the Kelvin limit. Predicted activation probability curves versus size (supersaturation) are steep, whence stringent experimental definitions of the thermodynamic state and the seed particle are required for meaningful comparison with theory. Activation curves for mobility-selected WOx particles are broader than predicted, even with a well-defined supersaturation, while those of mobility-purified molecular ions agree qualitatively with theory, even in a turbulent mixing nucleation chamber. Recent work by CitationWinkler (2009) based on the Vienna expansion chamber and mobility-purified molecular ions has anticipated these conclusions. The theory is combined with similar considerations on the onset of homogeneous nucleation, to draw conclusions on the smallest nucleus size that may be activated by heterogeneous nucleation. Water is predicted to be able to detect uncharged nuclei with diameters as small as 0.6 nm. The associated possibility to develop detectors for relatively small single neutral molecules is enticing." @default.
• W2053184447 created "2016-06-24" @default.
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• W2053184447 date "2011-03-10" @default.
• W2053184447 modified "2023-10-14" @default.
• W2053184447 title "Heterogeneous Nucleation with Finite Activation Energy and Perfect Wetting: Capillary Theory Versus Experiments with Nanometer Particles, and Extrapolations on the Smallest Detectable Nucleus" @default.
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• W2053184447 doi "https://doi.org/10.1080/02786826.2010.550341" @default.
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