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- W2053275311 abstract "Precision control of vapourization, both in space and time, has many potential applications; however, the physical mechanisms underlying controlled boiling are not well understood. The reason is the combined microscopic length scales and ultrashort timescales associated with the initiation and subsequent dynamical behaviour of the vapour bubbles formed. Here we study the nanoseconds vapour bubble dynamics of laser-heated single oil-filled microcapsules using coupled optical and acoustic detection. Pulsed laser excitation leads to vapour formation and collapse, and a simple physical model captures the observed radial dynamics and resulting acoustic pressures. Continuous wave laser excitation leads to a sequence of vapourization/condensation cycles, the result of absorbing microcapsule fragments moving in and out of the laser beam. A model incorporating thermal diffusion from the capsule shell into the oil core and surrounding water reveals the mechanisms behind the onset of vapourization. Excellent agreement is observed between the modelled dynamics and experiment. Laser-induced vapourization has great potential in many applications, but the underlying physical mechanisms are not clear. Here, Lajoinie et al.study oil-filled polymer microcapsules using coupled optical and acoustic detection, and report new insights into the laser-activated processes." @default.
- W2053275311 created "2016-06-24" @default.
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- W2053275311 date "2014-04-22" @default.
- W2053275311 modified "2023-10-18" @default.
- W2053275311 title "Ultrafast vapourization dynamics of laser-activated polymeric microcapsules" @default.
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- W2053275311 doi "https://doi.org/10.1038/ncomms4671" @default.
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