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- W2053314422 abstract "Any interpretation of the dynamics in liquids requires understanding of fluctuating collective motions in the stationary limit. To this end, “eigen-states” are defined, named conformons. Conformons are to be considered as a new type of bosons. Their properties characterize the typical features of the dynamics in disordered systems. Eigen-energy and “eigen-entropy” are adjusted to each other to minimize the free energy of each mode (saturation). The whole conformon ensemble exhibits a photon statistics with a broad universal mode spectrum. Analogues of Stefan-Boltzmann's law and of Wien's displacements law are formulated. A crucial point of our treatment is that conformons should, in principle, only become excited above a system-typical temperature To (Vogel-Fulcher temperature). Equilibrium properties of supercooled liquids are necessarily related to To. Cp/Cv, of the conformon ensemble should, for example, show a typical ΔT3-dependence (ΔT=T-To). Experimental data give evidence in support of this behaviour. As a consequence of the excluded volume supercooled liquids already solidify about 30 to 40 degrees above To at least at the quasi-static glass temperature Tg. Relaxation in the glass transition regime of glass formers can fully be described if relaxation modes are connected to each conformon. The description covers a set of experiments so different like mechanical and dielectric relaxation or quasi-elastic light- and neutron scattering." @default.
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- W2053314422 date "1995-02-01" @default.
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- W2053314422 title "Thermodynamics, dynamics and relaxation in glass-forming liquids - the conformon concept" @default.
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- W2053314422 doi "https://doi.org/10.1002/masy.19950900104" @default.
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