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- W2053404711 abstract "Desorption induced by single and multiple electronic transitions is described by a reduced density matrix formulation in a discrete energy representation. The discrete energy basis is comprised of the eigenfunctions of the system Hamiltonian augmented by an asymptotic potential wall, and has a number of advantages over its coordinate counterpart, such as the minimization of the basis size. The Liouville–von Neumann equation of a Lindblad semigroup form is solved numerically using a short-time Chebyshev propagation scheme. The dynamics of NO photodesorption from metals is investigated with one-dimensional two-state models corresponding to both the Menzel–Gormer–Redhead and Antoniewicz mechanisms. Desorption stimulated by both weak cw and strong pulsed light sources are examined." @default.
- W2053404711 created "2016-06-24" @default.
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- W2053404711 date "1999-11-08" @default.
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- W2053404711 title "Dissipative quantum dynamics in discrete energy representation: Photon-stimulated desorption of NO from metals" @default.
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- W2053404711 doi "https://doi.org/10.1063/1.480220" @default.
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