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- W2053576656 abstract "The metallization of poly(ethylene terephthalate) (PET) by copper has been studied by photoelectron spectroscopy (x-ray and vacuum ultraviolet). The results are interpreted in the light of a valence-effective-Hamiltonian band-structure calculation on the PET polymeric chain and by comparison with earlier work on copper oxides. The theoretical valence-band density of states is in very good agreement with the photoelectron spectra of PET and allows us to present a detailed interpretation of the valence electronic structure of PET. Upon metallization, we find that, for low coverages (5ifmmodetimeselsetexttimesfi{}${10}^{14}$ Cu atoms/${mathrm{cm}}^{2}$) copper binds preferentially to the oxygen from the carbonyl (---C---O) and the ether (---C---O---) groups of the PET. At coverages near 7.5ifmmodetimeselsetexttimesfi{}${10}^{14}$ Cu atoms/${mathrm{cm}}^{2}$, the additional copper remains metallic and gives rise to a three-dimensional islandlike growth mode. The low reactivity towards PET stands in sharp contrast to the case of other transition metals, like Ti and Cr." @default.
- W2053576656 created "2016-06-24" @default.
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- W2053576656 date "1991-11-15" @default.
- W2053576656 modified "2023-10-09" @default.
- W2053576656 title "Photoemission study of the copper/poly(ethylene terephthalate) interface" @default.
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- W2053576656 doi "https://doi.org/10.1103/physrevb.44.10815" @default.
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