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• W2053753904 abstract "The EPR spectrum of cyclopentadienylchromium tricarbonyl has been detected in single crystals of the diamagnetic manganese analog at temperatures below 25 K. Its g and 53Cr hyperfine matrices have been assembled in the crystal-axis system of the host. Both tensors are orthorhombic and their principal axes are almost coincident: g = (1.9969, 2.0353, 2.1339); a53 = (3, 27, 44) MHz. The proximity of the principal directions of the maximum and intermediate values of these tensors to certain directions in the host crystal shows that the chromium center substitutes for CpMn(CO)3 with little or no deformation. The single unpaired electron in CpCr(CO)3 is believed to occupy an a′ orbital (in Cs symmetry) which is composed of dx2−y2 and dyz chromium atomic orbitals, z being the molecular axis which connects Cr to the centers of Cp and the three CO ligands." @default.
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• W2053753904 date "1987-08-01" @default.
• W2053753904 modified "2023-09-27" @default.
• W2053753904 title "The EPR spectrum of CpCr(CO)3 in a single crystal of CpMn(CO)3 at 20 K" @default.
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• W2053753904 doi "https://doi.org/10.1016/0022-2364(87)90080-1" @default.
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