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- W2053806909 abstract "We present a microscopic description of the vibrational spectroscopy of the OH stretch of HOD in liquid D2O. Our model predicts that OH frequency correlations decay with a sharp and rapid (≈35 fs) decrease, followed by a beat at ≈125 fs from intermolecular oxygen vibrations. On a short time scale (≈200 fs), ultrafast infrared spectroscopy of the OH stretch is sensitive to localized intermolecular motions. For times longer than ≈200 fs, cooperative molecular rearrangements drive dephasing. The interplay of electric field fluctuations, both local and cooperative, dictate vibrational frequency shifts and destroy vibrational coherence in water." @default.
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- W2053806909 date "2005-09-30" @default.
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- W2053806909 title "Electric Field Fluctuations Drive Vibrational Dephasing in Water" @default.
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- W2053806909 doi "https://doi.org/10.1021/jp051364m" @default.
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