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• W2054181083 abstract "In rare gas matrices, gauche-Si4Me10 and trans-Si4Me10 have distinct IR and very different UV spectra, permitting selective phototransformation of one or the other into Si3Me8 and SiMe2 with monochromatic light, and separation of the spectra. t-Si4Me10 shows the expected red-shift relative to Si3Me8, but g-Si4Me10 does not. The consequences of this observation for simple theories of σ-conjugation are analyzed and an extension of the popular Sandorfy C model is proposed. Implications for conformationally induced segmentation of polysilane chains into weakly interacting chromophores are noted." @default.
• W2054181083 created "2016-06-24" @default.
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• W2054181083 date "1992-10-01" @default.
• W2054181083 modified "2023-09-27" @default.
• W2054181083 title "Conformational effects on σ-conjugation. UV and IR spectra of matrix-isolated trans- and gauche-n-Si4Me10" @default.
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• W2054181083 doi "https://doi.org/10.1016/0009-2614(92)85072-i" @default.
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