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- W2054328185 abstract "Nuclear materials used in the nuclear energy fuel cycle emit γ and self-excited x-rays. The fluorescent x-rays are excited by the material's own radiations and their intensities are stroingly correlated with the concentrations (mass fractions) of the corresponding chemical elements. The single measurement γ- and x-ray spectrum can be used not only to determine isotopic ratios but also for determination of plutonium and/or uranium concentrations. The proposed method uses the ratio of counting rates of plutonium K x-rays to 241Pu γ-rays as a measure of the sample's Pu concentration. This ratio is intrinsically calibrated: (i) it is corrected for the overall detecting efficiencies of γ- and x-rays; (ii) it is normalized for the isotopic composition of the measured sample and the isotopic ratios are determined from the same spectrum. Thus the number of required standards is minimal. For a narrow range of Pu concentrations only one standard is sufficient. The method has wide range of applications and potential to be highly accurate." @default.
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- W2054328185 date "1993-03-01" @default.
- W2054328185 modified "2023-09-23" @default.
- W2054328185 title "Intrinsically calibrated gamma and x-ray measurements of plutonium" @default.
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- W2054328185 doi "https://doi.org/10.1016/0969-8043(93)90178-d" @default.
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