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- W2054664335 abstract "Abstract The purpose of this work is to determine the partial molal quantities for the dissolution of nitrogen in nitrogen-rich α-U 2 N 3+ x in the low temperature range of 300–500°C where no thermodynamic data is available. α-U 2 N 3+ x with a high nitrogen content was prepared by reaction of UH 3 and an NH 3 + H 2 gas stream. The nitrogen activity a N , in the gas phase was controlled by changing the composition of the reactant gas. It was confirmed that N/U atom ratio of the sesquinitride varied when the composition of the reactant gas changed, which means that a N is dependent on the equilibrium nitrogen pressure of nitrogen-rich α-U 2 N 3+ x . This dependence was evaluated using the calculated value of a N . A composition-pressure-temperature relationship of the nitride phase is presented. The partial molal free energy, heat and entropy are calculated as a function of the composition." @default.
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- W2054664335 date "1996-01-01" @default.
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- W2054664335 title "Thermodynamic study of the dissolution of nitrogen in nitrogen-rich α-U2N3+" @default.
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- W2054664335 doi "https://doi.org/10.1016/0925-8388(95)01953-7" @default.
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