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- W2054838521 abstract "We demonstrate that photochromic molecules enable switching from the weak- to ultrastrong-coupling regime reversibly, by using all-optical control. This switch is achieved by photochemically inducing conformational changes in the molecule. Remarkably, a Rabi splitting of 700 meV is measured at room temperature, corresponding to 32% of the molecular transition energy. A similar coupling strength is demonstrated in a plasmonic structure. Such systems present a unique combination of coupling strength and functional capacities." @default.
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- W2054838521 date "2011-05-11" @default.
- W2054838521 modified "2023-10-04" @default.
- W2054838521 title "Reversible Switching of Ultrastrong Light-Molecule Coupling" @default.
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- W2054838521 doi "https://doi.org/10.1103/physrevlett.106.196405" @default.
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