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• W2054883931 abstract "We used dynamic 1 H NMR spectroscopic methods to examine the kinetics and thermodynamics of CH 3 CCl 3 ( 2 ) entering and leaving the gated molecular basket 1 . We found that the encapsulation is first-order in basket 1 and guest 2 , while the decomplexation is zeroth-order in the guest. Importantly, the interchange mechanism in which a molecule of CH 3 CCl 3 directly displaces the entrapped CH 3 CCl 3 was not observed. Furthermore, the examination of the additivity of free energies characterizing the encapsulation process led to us to deduce that the revolving motion of the gates and in/out trafficking of guests is synchronized, yet still a function of the affinity of the guest for occupying the basket: Specifically, the greater the affinity of the guest for occupying the basket, the less effective the gates are in “sweeping” the guest as the gates undergo their revolving motion." @default.
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• W2054883931 date "2012-01-16" @default.
• W2054883931 modified "2023-10-17" @default.
• W2054883931 title "On the mechanism of action of gated molecular baskets: The synchronicity of the revolving motion of gates and in/out trafficking of guests" @default.
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• W2054883931 doi "https://doi.org/10.3762/bjoc.8.9" @default.
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