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• W2054998668 startingPage "195" @default.
• W2054998668 abstract "Optimal control theory (OCT) is applied to laser cooling of molecules. The objective is to cool vibrations, using shaped pulses synchronized with the spontaneous emission. An instantaneous in time optimal approach is compared to solution based on OCT. In both cases the optimal mechanism is found to operate by a “vibrationally selective coherent population trapping”. The trapping condition is that the instantaneous phase of the laser is locked to the phase of the transition dipole moment of v=0 with the excited population. The molecules that reach v=0 by spontaneous emission are then trapped, while the others are continually repumped. For vibrational cooling to v=2 and rotational cooling, a different mechanism operates. The field completely changes the transient eigenstates of the Hamiltonian creating a superposition composed of many states. Finally this superposition is transformed by the field to the target energy eigenstate." @default.
• W2054998668 created "2016-06-24" @default.
• W2054998668 creator A5005564351 @default.
• W2054998668 creator A5046658383 @default.
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• W2054998668 date "2001-06-01" @default.
• W2054998668 modified "2023-10-15" @default.
• W2054998668 title "Laser cooling of molecules by dynamically trapped states" @default.
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• W2054998668 doi "https://doi.org/10.1016/s0301-0104(01)00266-x" @default.
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