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• W2055264889 endingPage "2812" @default.
• W2055264889 startingPage "2804" @default.
• W2055264889 abstract "The kinetics of the reduction of Fe(bipy)33+ by Co(dmgBF2)2(H2O)2 in 0.041 M HNO3/NaNO3 was found to be first-order in both the oxidizing and reducing agents and the second-order rate constant is given by kobs = k1 + k2K[Cl−], with k1=1.59 × 106 M−1 s−1and k2K = 1.83 × 108 M−2 s−1, at 25 °C. The term that is first-order in [Cl−] is attributed to the formation of an ion-pair between Fe(bipy)33+ and Cl−. For k1, the activation parameters ΔH* and ΔS* are 2.22 ± 0.02 kcal mol−1 and −22.7 ± 0.8 cal mol−1 K−1, respectively. The self-exchange rate constant of k22 ≈ 8.7 × 10−3 M−1 s−1 for Co(dmgBF2)2(H2O)2+/0 was estimated using Marcus theory and the known self-exchange rate constant for Fe(bipy)33+/2+." @default.
• W2055264889 created "2016-06-24" @default.
• W2055264889 creator A5055240446 @default.
• W2055264889 creator A5089444540 @default.
• W2055264889 date "2005-06-01" @default.
• W2055264889 modified "2023-10-18" @default.
• W2055264889 title "Kinetic studies of tris(2,2′-bipyridine)iron(III) perchlorate with cobaloxime, [Co(dmgBF2)2(H2O)2]" @default.
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• W2055264889 doi "https://doi.org/10.1016/j.ica.2005.03.001" @default.
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