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• W2055267319 startingPage "6178" @default.
• W2055267319 abstract "The electronic spectrum of thin films of poly(p-phenylene vinylene) (PPV) in an insulating neutral form exhibits three absorption bands with maxima at 6.12, 5.06, and 3.08 eV. The first two maxima are related to localized molecular states and the broad band at 3.08 eV is described in terms of a vibrationally coupled exciton model. Upon electrochemical doping of PPV, two additional absorption bands appear at 0.80 and 2.10 eV which are associated with a dication whose charge is spread over a few monomer units. Thin films of PPV can be electrochemically converted from the oxidized (conducting) form to the neutral (insulating) form repeatedly in LiAsF6/propylene carbonate solution without evidence of decomposition. The E0 measured using cyclic voltammetry is 3.85 V vs a Li/Li+ reference electrode; however, the observed optically active defects occur in a region of higher potential." @default.
• W2055267319 created "2016-06-24" @default.
• W2055267319 creator A5051329880 @default.
• W2055267319 creator A5080853404 @default.
• W2055267319 date "1987-11-15" @default.
• W2055267319 modified "2023-10-18" @default.
• W2055267319 title "Defects in the electronic structure of poly (<i>p</i>‐phenylene vinylene): Electronic spectra, electrochemical behavior, and molecular orbital calculations" @default.
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• W2055267319 doi "https://doi.org/10.1063/1.453493" @default.
• W2055267319 hasPublicationYear "1987" @default.
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