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- W2055351788 abstract "Time-resolved Raman probing technique is used to investigate the collisional relaxation of high-lying C-H vibrations in CHF 3 and CHF 2 Cl molecules. The relaxation rates both in collisions with parent molecules and a number of buffer gases were measured. The rate values were found to be abnormally fast. The relaxation is faster than single collision in parent gas and requires a few (3-8) collisions for nonpolar gases. For polar gases the relaxation is still faster. The conclusion is made that observed ultrafast relaxation of C-H modes is caused by energy transfer from excited «bright» states to nearby «dark» ones. Possible mechanisms of the above transfer are discussed" @default.
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- W2055351788 date "1995-03-01" @default.
- W2055351788 modified "2023-09-25" @default.
- W2055351788 title "Ultrafast Collisional Redistribution of Vibrational Energy in Highly Excited Polyatomic Molecules. The Role of Intramolecular Interactions" @default.
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- W2055351788 doi "https://doi.org/10.1002/bbpc.19950990320" @default.
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