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• W2055430830 endingPage "8820" @default.
• W2055430830 startingPage "8813" @default.
• W2055430830 abstract "We report the synthesis of a series of amphiphilic molecular building blocks that can be self-assembled at the air-water interface to form two- and three-dimensional nanostructures with tunable optoelectronic properties. Compression of these molecular building blocks using the Langmuir-Blodgett method gives rise to monolayer and multilayer thin films with different packing densities and electronic properties that are tunable due to varying pi-pi (hydrophobic) interactions. Depending on the noncovalent interaction between chromophores, we observe a transition toward denser packing with increasing number of phenylene ethynylene repeat units. Additionally, we use quantum-chemical simulations to help determine the excited-state electronic structure, intermolecular interactions, and packing trends. Our results demonstrate that the interplay between dipole-dipole and pi-pi interactions dominates the formation of thin films with various packing densities and determines the associated optical properties." @default.
• W2055430830 created "2016-06-24" @default.
• W2055430830 creator A5056150849 @default.
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• W2055430830 date "2006-09-06" @default.
• W2055430830 modified "2023-09-25" @default.
• W2055430830 title "Synthesis and Characterization of Amphiphilic Phenylene Ethynylene Oligomers and Their Langmuir−Blodgett Films" @default.
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• W2055430830 doi "https://doi.org/10.1021/la060914k" @default.
• W2055430830 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/17014122" @default.
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