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- W2055497044 abstract "Electron paramagnetic resonance measurements of ${mathrm{NiCl}}_{2}ensuremath{-}4mathrm{SC}({mathrm{NH}}_{2}{)}_{2}$ reveal the low-energy spin dispersion, including a magnetic-field interval in which the two-magnon continuum is within ${k}_{B}T$ of the ground state, allowing a continuum of excitations over a range of $k$ states, rather than only the $k=0$ single-magnon excitations. This produces a novel $Y$ shape in the frequency-field EPR spectrum measured at $Tensuremath{ge}1.5text{ }text{ }mathrm{K}$. Since the interchain coupling ${J}_{ensuremath{perp}}ensuremath{ll}{k}_{B}T$, this shape can be reproduced by a single $S=1$ antiferromagnetic Heisenberg chain with a strong easy-plane single-ion anisotropy. Importantly, the combination of experiment and modeling we report herein demonstrates a powerful approach to probing spin dispersion in a wide range of interacting magnetic systems without the stringent sample requirements and complications associated with inelastic scattering experiments." @default.
- W2055497044 created "2016-06-24" @default.
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- W2055497044 date "2008-08-21" @default.
- W2055497044 modified "2023-09-27" @default.
- W2055497044 title "Unusual Magneto-Optical Phenomenon Reveals Low Energy Spin Dispersion in the Spin-1 Anisotropic Heisenberg Antiferromagnetic Chain SystemNiCl2−4SC(NH2)2" @default.
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- W2055497044 doi "https://doi.org/10.1103/physrevlett.101.087602" @default.
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