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- W2055767784 endingPage "10347" @default.
- W2055767784 startingPage "10338" @default.
- W2055767784 abstract "Electropolymerization, morphology characterization, and ion transport of poly(3,4-ethylenedioxythiophene) (PEDOT) films doped with different counterions (chloride, ferrocyanide (FCN), and poly(p-styrenesulfonate) (PSS-)) on a platinum electrode were investigated using scanning electrochemical microscopy (SECM) during both potential step (chronocoulometric) and cyclic voltammetric scans. An ultramicroelectrode (UME) tip was positioned close to the surface of a PEDOT-modified substrate electrode, and the responses of both electrodes to a substrate potential step or linear sweep were monitored simultaneously. Chloride or ferrocyanide (FCN) ejection during PEDOT reduction was shown to be a function of the reduction potential. The nature of the cation in the bulk solution was not found to be important in the kinetics of ion transport in PEDOT+/FCN- films. Direct evidence for the incorporation of cations of Ru(NH3)6(3+/2+) in a PEDOT film during its reduction was also obtained by SECM measurements. The adsorption of Ru(NH3)6(3+) in fully oxidized PEDOT+/PSS- films was observed and attributed to ion exchange between the Na+ co-ion of PSS- and Ru(NH3)6(3+) in the bulk solution." @default.
- W2055767784 created "2016-06-24" @default.
- W2055767784 creator A5003590706 @default.
- W2055767784 creator A5070242592 @default.
- W2055767784 date "2006-08-25" @default.
- W2055767784 modified "2023-10-18" @default.
- W2055767784 title "Polymer Films on Electrodes: Investigation of Ion Transport at Poly(3,4-ethylenedioxythiophene) Films by Scanning Electrochemical Microscopy" @default.
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