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- W2055919645 abstract "Semiconductor/electrolyte model interfaces are prepared in UHV by coadsorbing the redox active electrolyte species Br2 and the solvent H2O onto chemically inert van der Waals (0001) surfaces of WSe2. Only a small fraction of the adsorbed Br2 is ionosorbed due to charge exchange with the semiconductor bulk; most of it and H2O are molecularly adsorbed. Thus the observed changes of band bending and work function are related to charge transfer processes at the interface to achieve electronic equilibrium. The value of band bending obtained for the model electrolyte is in reasonable agreement to the equivalent Volta potential of the electrolyte contact. For the Br2/H2O coadsorption system it is only determined by Br2 and not affected by coadsorbed H2O. In addition, the relative density of state distribution of the semiconductor and the model electrolyte can directly be determined from the electron distribution curve of the valence band region and compared to theoretical expectations of electrolyte interfaces. W..." @default.
- W2055919645 created "2016-06-24" @default.
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- W2055919645 date "1996-01-01" @default.
- W2055919645 modified "2023-09-27" @default.
- W2055919645 title "Synchrotron-Induced Photoelectron Spectroscopy of Semiconductor/Electrolyte Model Interfaces: Coadsorption of Br2 and H2O on WSe2(0001)" @default.
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- W2055919645 doi "https://doi.org/10.1021/jp961116d" @default.
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