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- W2055975707 abstract "Polarized optical spectroscopy has been used to investigate the electronic structure of tetravalent neptunium incorporated as a dilute impurity in single crystals of the tetragonal host ${mathrm{ZrSiO}}_{4}$. Thirty-one levels were assigned from 30 intense polarized optical transitions and used to obtain a fit to a parametric Hamiltonian to within an rms deviation of 34 ${mathrm{cm}}^{mathrm{ensuremath{-}}1}$. Thirteen other levels with comparable intensities and good polarization characteristics were observed. Inclusion of these levels using the parameters from the 31-level fit, however, resulted in an increase of the rms deviation to approximately 100 ${mathrm{cm}}^{mathrm{ensuremath{-}}1}$. The EPR spectra of the ground state of ${mathrm{Np}}^{4+}$:${mathrm{ZrSiO}}_{4}$ were measured and fit to an axial spin Hamiltonian to obtain the parameters: ensuremath{Vert}${g}_{?}$ensuremath{Vert}=0.8ifmmodepmelsetextpmfi{}0.6, ensuremath{Vert}${g}_{ensuremath{perp}}$ensuremath{Vert}=2.59ifmmodepmelsetextpmfi{}0.02, A=-2400ifmmodepmelsetextpmfi{}1200 MHz, and B=4750ifmmodepmelsetextpmfi{}30 MHz. These results are consistent with the calculated ${ensuremath{Gamma}}_{6}$ ground state." @default.
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- W2055975707 date "1988-03-01" @default.
- W2055975707 modified "2023-09-25" @default.
- W2055975707 title "Optical and EPR investigations ofNp4+in single crystals ofZrSiO4" @default.
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- W2055975707 doi "https://doi.org/10.1103/physrevb.37.3255" @default.
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