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• W2056005403 abstract "Abstract The S 1 –S 0 resonant enhanced multiphoton ionization (REMPI) spectrum as well as the infrared (IR) spectra in the S 0 and S 1 states of 4‐aminobenzonitrile (4ABN) and its van der Waals complex with Ar (4ABN–Ar) were measured by means of IR depletion spectroscopy (REMPI–IR). The IR spectrum of 4ABN–Ar in S 0 shows symmetric and antisymmetric NH stretching vibrations ( ν s and ν a ) of the amino group at the same positions as those in the 4ABN monomer. This suggests that the Ar ligand locates above the benzene ring by van der Waals interactions (π‐bound). The same coincidence of vibrational frequencies was found in S 1 , and the π‐bound geometry was kept by the electronic excitation. The REMPI–IR spectrum of 4ABN + –Ar was also measured, and three major vibrational transitions were found. From the comparison to the IR dissociation spectrum with an electron impact source (EI–IR), they were assigned to ν s , ν a and an NH‐bending overtone of the π‐bound structure. It is concluded that photoionization of 4ABN + –Ar does not promote site‐switching of Ar from the π‐site to the H‐site." @default.
• W2056005403 created "2016-06-24" @default.
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• W2056005403 date "2012-11-26" @default.
• W2056005403 modified "2023-10-17" @default.
• W2056005403 title "IR Spectroscopy of the 4‐Aminobenzonitrile–Ar Cluster in the S₀, S₁ Neutral and D₀ Cationic States" @default.
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• W2056005403 doi "https://doi.org/10.1002/cphc.201200821" @default.
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