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- W2056510313 abstract "Thermodynamic activity of SrO, aSrO, in lanthanum manganite doped with SrO with the stoichiometry La1−xSrxMnO3−y (where x=0.065, 0.10, 0.15 or 0.20) was measured as a function of temperature over the range of ∼750–1000 K by employing an EMF technique with CaF2 or SrF2 as the fluoride ion conducting electrolyte under an atmosphere of oxygen at unit fugacity. When Pt/SrO,SrF2,O2 was used as the reference electrode for the test electrode Pt/0.15 LSM, SrF2,O2, sintered SrF2 was used as the electrolyte. In all other galvanic cells, both the test and reference electrodes contained LSM with different dopant concentrations. The SrO potential ΔGSrO, log aSrO and the corresponding activity coefficients (γSrO) for the four solid solutions were determined and log aSrO was found to exhibit decreasing negative deviation from ideality with increasing SrO content. The ΔGSrO for these compositions could be represented as −4.81–0.03360T (K) for 0.065 LSM, −5.68–0.02818T for 0.10 LSM, −9.84–0.01950T for 0.15 LSM and −11.42–0.01360T for 0.20 LSM in terms of kJ mol−1." @default.
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- W2056510313 date "2001-06-01" @default.
- W2056510313 modified "2023-10-16" @default.
- W2056510313 title "Activity of SrO in La1−xSrxMnO3−y (x=0.065, 0.10, 0.15 or 0.20) by a solid state EMF method" @default.
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- W2056510313 doi "https://doi.org/10.1016/s0925-8388(01)01215-4" @default.
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