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- W2056510452 abstract "We theoretically study the photoinduced ionic→neutral phase transition in the quasi-one-dimensional molecular crystal TTF-CA. Our theoretical model includes strong intra-chain Coulomb interactions as well as very weak inter-chain interactions. Within the mean-field picture, we investigate the nonlinear lattice relaxation of a charge transfer exciton, and clarify the adiabatic path from its Franck-Condon state to a macroscopic neutral domain. It is found that the lowest state of such a single charge transfer exciton can not relax down to the neutral domain straightly, but a large excess energy is necessary so that it can overcome a high barrier. The aggregation of two identically shaped neutral domains is also discussed." @default.
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- W2056510452 date "2001-12-10" @default.
- W2056510452 modified "2023-09-27" @default.
- W2056510452 title "THEORY OF PHOTOINDUCED PHASE TRANSITION IN THE QUASI-ONE-DIMENSIONAL CHARGE TRANSFER COMPOUND TTF-CA" @default.
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- W2056510452 doi "https://doi.org/10.1142/s0217979201008494" @default.
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