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• W2056546702 abstract "The reactivity of different nitrogen-containing compounds, which may be formed as intermediates during the selective catalytic reduction of nitrogen oxides with organic compounds over alumina (HC-SCR), has been investigated in the temperature range of 60–610°C in a flow reactor system equipped with an FTIR gas analyzer. Tert-butylnitrile N-oxide (t-CNO), t-butyl isocyanate (t-NCO) and t-butyl cyanide (t-CN) were used as model compounds. The reactivity tests comprised the decomposition and oxidation reactions in a stream of O2 and N2, and in mixtures of NO2 or NO with O2 (HC-SCR conditions). These studies revealed that t-CNO isomerizes readily to t-NCO and then decomposes to CO2 and t-butylamine. The latter rapidly reacts with NO2 to form N2 or further decomposes into isobutene and NH3, which may be followed by the conventional SCR with NH3 as a reducing agent. This suggests that once nitrile N-oxides are formed under HC-SCR conditions they are readily converted to N2 through several reaction steps." @default.
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• W2056546702 date "1998-10-01" @default.
• W2056546702 modified "2023-10-10" @default.
• W2056546702 title "Reactivity of nitrogen containing organic intermediates in the selective catalytic reduction of NOx with organic compounds: a model study with tert-butyl substituted nitrogen compounds" @default.
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• W2056546702 doi "https://doi.org/10.1016/s0926-3373(98)00053-8" @default.
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