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- W2056552544 abstract "Abstract The first three-dimensional quantum-dynamical ab initio simulation of the large amplitude vibrational dynamics of an Ag 3 cluster initiated from its linear transition state is presented. This can be monitored by femtosecond pump-probe negative-ion to neutral-to-positive-ion spectroscopy with zero electron kinetic energy (NeNePo-ZEKE). The time evolution of the representative wavepacket confirms the dynamical effects which have been discovered previously by Wigner-type semiclassical simulations: the initial coherent bending and stretching from linear to near equilateral triangular configuration, followed by intracluster collision and intracluster vibrational relaxation with a weak fractional revival. In addition, the quantum wavepacket shows interferences and spreading." @default.
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- W2056552544 date "2000-02-01" @default.
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- W2056552544 title "Ab initio three-dimensional quantum dynamics of Ag3 clusters in the NeNePo process" @default.
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- W2056552544 doi "https://doi.org/10.1016/s0009-2614(00)00027-0" @default.
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