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- W2056553899 abstract "The concept of a substrate length L is essential in the understanding of the regime I→II growth rate transitions in melt-crystallized lamellar polymers. The present work deals with the actual magnitude of L in polyethylene fractions as determined strictly from the kinetics of crystallization. With the help of an improved value of the activation energy of transport in the melt, and a more precise method of analysis than was employed heretofore, it is found from published growth rate measurements on polyethylene fractions that L is within about a factor of two of 0.77 μm at the regime I→II transition. The value of L is independent of the equilibrium melting temperature T0m(∞) assumed in the analysis. It is shown that L is much larger than a just stable surface nucleus. A brief summary is given of what is known about L from a kinetic point of view, and possible correlations with morphological features are mentioned. It is conjectured that L may relate to the mean distance between surface defects that have the capacity to terminate strip completion. In the course of the study, better values of the pre-exponential factors N0 and C0 that govern the absolute growth rates in regimes I and II, respectively, are obtained. A revised numerical value is given for the pre-exponential factor in the Lauritzen ‘Z’ test. This is based partly on the new value of C0, and partly on a reformulation of the problem." @default.
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- W2056553899 date "1985-06-01" @default.
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- W2056553899 title "The kinetic substrate length in nucleation-controlled crystallization in polyethylene fractions" @default.
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- W2056553899 doi "https://doi.org/10.1016/0032-3861(85)90121-1" @default.
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