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• W2056556970 abstract "N-Heterocyclic carbenes (NHCs) catalyze a domino Michael addition/acylation reaction to form 3,4-dihydrocoumarins. The reaction proceeds through addition of the NHC to an aryloxyaldehyde followed by elimination of a phenoxide leaving group, generating an enol intermediate. This transient nucleophile generated in situ performs a 1,4-addition onto a conjugate acceptor, and the carbene catalyst is regenerated upon acylation of the phenoxide anion resulting in formation of 3,4-dihydrocoumarins." @default.
• W2056556970 created "2016-06-24" @default.
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• W2056556970 date "2008-12-02" @default.
• W2056556970 modified "2023-09-27" @default.
• W2056556970 title "NHC-Catalyzed Reactions of Aryloxyacetaldehydes: A Domino Elimination/Conjugate Addition/Acylation Process for the Synthesis of Substituted Coumarins" @default.
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• W2056556970 doi "https://doi.org/10.1021/ol802448c" @default.
• W2056556970 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/2640423" @default.
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