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• W2056557065 endingPage "3588" @default.
• W2056557065 startingPage "3577" @default.
• W2056557065 abstract "The three-component irreversible surface-reaction model A+BCensuremath{rightarrow}AC+1/2${mathit{B}}_{2}$ with infinite reaction rates between nearest-neighbor adspecies is studied by Monte Carlo simulations. For a square lattice the system evolves to a degenerate poisoned state exponentially in time, except for a narrow range of pressures in which a reactive quasi-steady-state exists. The latter poisons very slowly in time. For a hexagonal lattice a true reactive steady state occurs for a range of pressures bordered by continuous and discontinuous transitions to poisoned states. The latter behavior is observed by adding the reaction channel A+Bensuremath{rightarrow}AB on a square lattice. Some properties of these models are elucidated by analysis of appropriate exact master equations and corresponding pair approximations. Other issues addressed include ``extent of variability'' of the degenerate poisoned states, the effect of finite reaction rates, and spatial correlations." @default.
• W2056557065 created "2016-06-24" @default.
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• W2056557065 date "1993-11-01" @default.
• W2056557065 modified "2023-09-27" @default.
• W2056557065 title "Transitions in the kinetics and steady states of irreversible<i>A</i>+<i>BC</i>surface-reaction models" @default.
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• W2056557065 doi "https://doi.org/10.1103/physreve.48.3577" @default.
• W2056557065 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/9961015" @default.
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