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- W2056564487 abstract "Fluorescence lifetimes of the single vibronic levels of the first excited singlet states of H2CS, D2CS and Cl2CS have been measured under effusive flow conditions. The single exponential lifetimes of H2CS (D2CS) decrease from 140 μs (182 μs) to 72 μs (95 μs) with increasing vibrational levels of Ā1A2 state. At the same excitation energy, the lifetime of H2CS (Ā1A2) is shorter than that of D2CS (Ā1A2). The difference is attributed to a tunnelling effect in a non-radiative process. The decay of Cl2CS(̄A1A2) is not single exponential. Assuming a bi-exponential decay, the shorter fluorescence lifetime decreases with the vibrational levels, while the longer one increases. The difference between H2CS and Cl2CS is discussed in terms of non-radiative processes including dissociation and intersystem crossing." @default.
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- W2056564487 date "1985-03-01" @default.
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- W2056564487 title "Fluorescence lifetimes of the single vibrational levels of H2CS1, D2CS, and Cl2CS in the Ā1A2 state" @default.
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- W2056564487 doi "https://doi.org/10.1016/0301-0104(85)85075-8" @default.
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