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- W2056565592 abstract "Sulphur capture by lime was studied in a 16 MW stationary fluidized bed boiler (FBB). A marked fall-off in sulphur capture was noted at temperatures above about 880 °C. The proposed explanation is that the combustion produces reducing conditions in the particle phase, and thus allows for a reductive decomposition of CaSO4. This explanation is supported by (i) thermodynamics showing the instability of CaSO4 under reducing conditions; (ii) in-bed oxygen measurements indicating reducing conditions in the particle phase; (iii) the observed fall-off in sulphur capture with temperature, which is not seen in laboratory tests under oxidizing conditions or in a circulating FBB, where the sorbent particles experience oxidizing conditions to a greater extent; (iv) the observation that the temperature dependence of the sulphur emission is very strong even when the net sulphur capture is zero provided always that CaSO4 is present and (v) literature data indicating the rate of the proposed reaction." @default.
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- W2056565592 date "1989-03-01" @default.
- W2056565592 modified "2023-09-27" @default.
- W2056565592 title "Sulphur capture in fluidized bed boilers: The effect of reductive decomposition of CaSO4" @default.
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- W2056565592 doi "https://doi.org/10.1016/0300-9467(89)80047-4" @default.
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