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• W2056588194 abstract "A theory of desorption induced by an infrared laser is developed. The laser excites a molecule to the first excited level and higher vibrational levels are excited by the intermolecular energy transfer. Once the molecule is excited to the higher levels it might desorb. The theory of this process includes a derivation, from “first principles”, of corresponding master equations. These equations include both usual distribution functions and pair distribution functions. It is shown that a frequency dependence of the yield from the Rth excited level is determined by the Rth degree of the corresponding Lorentzian. This yield is also proportional to Rth degree of the laser field intensity." @default.
• W2056588194 created "2016-06-24" @default.
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• W2056588194 date "1986-03-01" @default.
• W2056588194 modified "2023-10-17" @default.
• W2056588194 title "Theoretical studies of laser-stimulated surface processes III: Effect of vibrational energy transfer on desorption" @default.
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• W2056588194 doi "https://doi.org/10.1016/0378-4363(86)90493-6" @default.
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