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- W2056734695 abstract "Thiol additions to the highly functionalized core structures of aranorosin- and manumycin-type antibiotics reveal the general reactivity patterns of epoxyketone natural products. Rapid hemiacetal and hydrate formations decrease the reactivity of the epoxyketone moiety in aqueous media toward the cellular scavenger glutathione, and secondary 1,2-shift, elimination, aromatization and intramolecular aldol reactions provide novel reaction pathways. In a hydrophobic environment, the thiol-capture function of the ketone moiety facilitates electrophilic attack." @default.
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- W2056734695 title "Thiophilic ring-opening and rearrangement reactions of epoxyketone natural products" @default.
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- W2056734695 doi "https://doi.org/10.1016/s0960-894x(98)00026-2" @default.
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