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- W2056777582 abstract "We report a study of the oxidation of CO on a gold nanotip in the presence of high electrostatic fields. With the binding energies obtained using density functional theory as a function of the electric field, a simple field-dependent kinetic model based on the Langmuir-Hinshelwood mechanism is set up. We show that the dissociative adsorption of oxygen on gold happens only below a negative critical value of the electric field while the binding of CO on gold is enhanced for positive values. We explain the propagation of a wave observed in field ion microscopy experiments and predict that the oxidation of CO occurs on negatively charged gold clusters." @default.
- W2056777582 created "2016-06-24" @default.
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- W2056777582 date "2006-12-06" @default.
- W2056777582 modified "2023-09-27" @default.
- W2056777582 title "CO oxidation on electrically charged gold nanotips" @default.
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- W2056777582 doi "https://doi.org/10.1063/1.2400035" @default.
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