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• W2056870085 abstract "Abstract The relaxation of H and D in Pd 90 Gd 5 Fe 5 was investigated over a wide temperature range by means of internal friction (IF) using a vibrating reed apparatus (frequencies 450 Hz…2100 Hz) and an inverted torsion pendulum (1 Hz…12 Hz) and by means of magnetic after-effect (MAE) (relaxation times corresponding to frequencies of 0.005 Hz…0.17 Hz). After charging with H, Pd 90 Gd 5 Fe 5 H 5.65 shows a relaxation maximum in the MAE at 68 K ( f >=0.005 Hz) and a maximum of the IF at 108 K ( f =4.7 Hz). The activation parameters were determined independently by both methods to τ 0 H =4·10 −12±0.5 s and H a H =(0.19±0.02) eV. With decreasing H or D content this maximum shifts to higher temperatures, similar to the shift in the binary alloy Pd 100− x Gd x . Owing to this concentration dependence, together with the similar activation parameters, the relaxation maximum can be attributed to the reorientation of H–Gd complexes. For identical concentrations, the IF relaxation maximum shows an isotope shift of about 5 K to lower temperatures for deuterium with respect to hydrogen. For a concentration of 3.85 at.%, activation parameters of τ 0 H =6·10 −12±0.5 s, H a H =(0.21±0.01) eV and τ 0 D =6·10 −13±0.5 s, H a D =(0.23±0.01) eV were obtained." @default.
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• W2056870085 date "1999-02-01" @default.
• W2056870085 modified "2023-09-25" @default.
• W2056870085 title "Mechanical and magnetic relaxation of H and D in dilute PdGdFe" @default.
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• W2056870085 doi "https://doi.org/10.1016/s0925-8388(98)00886-x" @default.
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