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• W2056930844 abstract "Iridium nanoparticles have only been reported with roughly spherical shapes and sizes of 1–5 nm, making it impossible to investigate their facet-dependent catalytic properties. Here we report for the first time a simple method based on seed-mediated growth for the facile synthesis of Ir nanocrystals with well-controlled facets. The essence of this approach is to coat an ultrathin conformal shell of Ir on a Pd seed with a well-defined shape at a relatively high temperature to ensure fast surface diffusion. In this way, the facets on the initial Pd seed are faithfully replicated in the resultant Pd@Ir core–shell nanocrystal. With 6 nm Pd cubes and octahedra encased by {100} and {111} facets, respectively, as the seeds, we have successfully generated Pd@Ir cubes and octahedra covered by Ir{100} and Ir{111} facets. The Pd@Ir cubes showed higher H2 selectivity (31.8% vs 8.9%) toward the decomposition of hydrazine compared with Pd@Ir octahedra with roughly the same size." @default.
• W2056930844 created "2016-06-24" @default.
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• W2056930844 date "2014-07-28" @default.
• W2056930844 modified "2023-10-06" @default.
• W2056930844 title "Facile Synthesis of Iridium Nanocrystals with Well-Controlled Facets Using Seed-Mediated Growth" @default.
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• W2056930844 doi "https://doi.org/10.1021/ja505716v" @default.
• W2056930844 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/25058427" @default.
• W2056930844 hasPublicationYear "2014" @default.
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