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- W2056945192 abstract "The interfacial temperature is important in gas absorption because it sets the solubility. If the gas undergoes an exothermic reaction this temperature ordinarily exceeds the bulk liquid temperature. For a bimolecular reaction the pseudo-first-order approximation leads to a serviceable model; yet it must overestimate the temperature rise under fast reaction conditions. We correct this estimate by accounting for the depletion of the liquid-phase reactant near the surface. To do this we use an enhancement factor based on the van Krevelen-Hoftijzer approximation. This implies a simple formula for the temperature rise not unlike that based on the pseudo-first-order approximation. We investigate this formula and show that it exhibits either one or three solutions. We deduce criteria for predicting, a priori, both what the multiplicity is and whether or not the maximum temperature rise corresponding to instantaneous reaction obtains." @default.
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- W2056945192 date "1986-11-01" @default.
- W2056945192 modified "2023-09-27" @default.
- W2056945192 title "THE DIFFUSIONAL LIMITATION ON THE TEMPERATURE RISE IN THE ABSORPTION OF CHEMICALLY REACTIVE GASES" @default.
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- W2056945192 doi "https://doi.org/10.1080/00986448608911785" @default.
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