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- W2057180010 abstract "The thermodynamic state of hydrogen in aluminum during alkaline corrosion was investigated, using a two-compartment hydrogen permeation cell with an Al/Pd bilayer membrane. The open-circuit potential of the Pd layer in a pH 7.0 buffer solution was monitored to sense the hydrogen chemical potential, μH. At pH 12.5–13.5, the measurements established a minimum μH of 0.55 eV relative to the ideal gas reference, equivalent to a H2 gas pressure of 5.7 GPa. Statistical mechanics calculations show that vacancy-hydrogen defects are stable in Al at this condition. A dissolution mechanism was proposed in which H at very high μH is produced by oxidation of interfacial aluminum hydride. The mechanism explains the observed rapid accumulation of H in the metal by extensive formation of vacancy-hydrogen defects." @default.
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- W2057180010 date "2010-07-01" @default.
- W2057180010 modified "2023-09-24" @default.
- W2057180010 title "Hydrogen in aluminum during alkaline corrosion" @default.
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- W2057180010 doi "https://doi.org/10.1016/j.electacta.2010.04.076" @default.
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