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- W2057183934 abstract "Poly(aryleneethynylene) type π-conjugated polymers (PAEs) are synthesized and the third-order optical susceptibility χ (3) of their thin films is evaluated. There is a red-shift in the electronic absorption of the PAE caused by an intramolecular charge transfer (CT) interaction when π-electron excessive heteroaromatic rings are introduced into the π-conjugation. The χ (3) value of the PAEs is enhanced by increasing the CT interaction and reaches more than 10 -11 esu in the near resonant region. The increase in the π-electron delocalization caused by the CT interaction is found to be the main factor enhancing χ (3) . This introduction of a CT interaction into a π-conjugation is an effective concept for the design of large χ (3) materials." @default.
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- W2057183934 date "1995-06-01" @default.
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- W2057183934 title "Enhancement of Third-Order Optical Nonlinearity of Poly(aryleneethynylene)s by Introducing an Intramolecular Charge Transfer Interaction into Their π-Conjugation" @default.
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- W2057183934 doi "https://doi.org/10.1143/jjap.34.3139" @default.
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