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• W2057358001 abstract "Laser-ablated yttrium and scandium metal atoms have been codeposited at 4 K with acetylene in excess argon. Products, Y(C(2)H(2)), HYCCH, HScCCH(-), and HScScCCH(-), have been formed in the present experiments and characterized using infrared spectroscopy on the basis of the results of the isotopic shifts, mixed isotopic splitting patterns, stepwise annealing, the change of reagent concentration and laser energy, and the comparison with theoretical predictions. Density functional theory calculations have been performed on these molecules. The agreement between the experimental and calculated vibrational frequencies, relative absorption intensities, and isotopic shifts supports the identification of these molecules from the matrix infrared spectra. Plausible reaction mechanisms have been proposed to account for the formation of these molecules." @default.
• W2057358001 created "2016-06-24" @default.
• W2057358001 creator A5064109029 @default.
• W2057358001 creator A5078769160 @default.
• W2057358001 date "2010-08-09" @default.
• W2057358001 modified "2023-10-16" @default.
• W2057358001 title "Reactions of Yttrium and Scandium Atoms with Acetylene: A Matrix Isolation Infrared Spectroscopic and Theoretical Study" @default.
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• W2057358001 doi "https://doi.org/10.1021/jp103486f" @default.
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