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• W2057382835 endingPage "4894" @default.
• W2057382835 startingPage "4888" @default.
• W2057382835 abstract "The ability of the modified electro-Fenton-like (EF-like) process to degrade aqueous solutions of glyphosate, which is the most widely used herbicide in the world, has been assessed with Mn2+ and other metal ions as catalysts to overcome the problems posed by some stable metal ion complexes of phosphonate herbicides. Bulk electrolyses with a carbon-felt cathode and Pt anode were performed in an undivided cell under galvanostatic conditions to study the effect of the applied current as well as Mn2+ and glyphosate concentrations. The herbicide was completely destroyed in all cases following a pseudofirst-order kinetics, and the second-order rate constant for its reaction with •OH was determined. The decay trends obtained by high-performance liquid chromatography−fluorometric detection (HPLC-FL) and ion chromatography analysis were similar. AMPA [(aminomethyl)phosphonic acid] was the major reaction intermediate and showed slower pseudofirst-order destruction kinetics. The high mineralization degree obtained for glyphosate solutions confirmed the great performance of the EF-like process with Mn2+, which promotes the C−N cleavage by •OH attack as the first oxidation step and the C−P cleavage in a further step. High-level decontamination achieved for AMPA and glufosinate solutions corroborated the benefits of this oxidation process." @default.
• W2057382835 created "2016-06-24" @default.
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• W2057382835 date "2009-05-13" @default.
• W2057382835 modified "2023-10-17" @default.
• W2057382835 title "Decontamination of Aqueous Glyphosate, (Aminomethyl)phosphonic Acid, and Glufosinate Solutions by Electro-Fenton-like Process with Mn²⁺ as the Catalyst" @default.
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• W2057382835 doi "https://doi.org/10.1021/jf900876x" @default.
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