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- W2057456499 abstract "A rigorous theoretical connection between the polarizability spectral density obtained from optical Kerr effect (OKE) measurement with the correlation function describing solvent-induced optical dephasing detected in photon echo measurements is given. The experimentally obtained spectral density has a more reasonable physical basis than model correlation function descriptions of solvent fluctuations. The experimental OKE spectrum is demonstrated to provide a natural description of solvent motions that modulate the chromophore electronic states in the case of weak induced-dipolar interactions. The chromophore optically active vibrational modes are obtained from pump-probe spectra and are employed in the calculation of echo signals. It is found that the fast decays of the two-pulse echo signals result from both solvent and solute intramolecular motions while the echo peak shifts are dominated by the solvent intermolecular modes." @default.
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- W2057456499 date "1995-11-15" @default.
- W2057456499 modified "2023-10-18" @default.
- W2057456499 title "The solvent spectral density and vibrational multimode approach to optical dephasing: Two-pulse photon echo response" @default.
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- W2057456499 doi "https://doi.org/10.1063/1.470147" @default.
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